• 文献标题:   Raman spectra and electron-phonon coupling in disordered graphene with gate-tunable doping
  • 文献类型:   Article
  • 作  者:   CHILDRES I, JAUREGUI LA, CHEN YP
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF APPLIED PHYSICS
  • ISSN:   0021-8979 EI 1089-7550
  • 通讯作者地址:   Purdue Univ
  • 被引频次:   14
  • DOI:   10.1063/1.4903959
  • 出版年:   2014

▎ 摘  要

We report a Raman spectroscopy study of graphene field-effect transistors with a controlled amount of defects introduced in graphene by exposure to electron-beam irradiation. Raman spectra are taken at T = 8 K over a range of back gate voltages (V-g) for various irradiation dosages (R-e). We study effects in the Raman spectra due to V-g-induced doping and artificially created disorder at various R-e. With moderate disorder (irradiation), the Raman G peak with respect to the graphene carrier density (n(FE)) exhibits a minimum in peak frequency and a maximum in peak width near the charge-neutral point (CNP). These trends are similar to those seen in previous works on pristine graphene and have been attributed to a reduction of electron-phonon coupling strength (D) and removal of the Kohn anomaly as the Fermi level moves away from the CNP. We also observe a maximum in I-2D/I-G and weak maximum in I-D/I-G near the CNP. All the observed dependences of Raman parameters on nFE weaken at stronger disorder (higher R-e), implying that disorder causes a reduction of D as well. Our findings are valuable for understanding Raman spectra and electron-phonon physics in doped and disordered graphene. (C) 2014 AIP Publishing LLC.