• 文献标题:   Direct Visualization of Native Defects in Graphite and Their Effect on the Electronic Properties of Bernal-Stacked Bilayer Graphene
  • 文献类型:   Article
  • 作  者:   JOUCKEN F, BENA C, GE ZH, QUEZADALOPEZ E, PINON S, KALADZHYAN V, TANIGUCHI T, WATANABE K, FERREIRA A, JR JV
  • 作者关键词:   bilayer graphene, graphite, scanning tunneling microscopy, quasiparticle interference, dopant
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984 EI 1530-6992
  • 通讯作者地址:  
  • 被引频次:   12
  • DOI:   10.1021/acs.nanolett.1c01442 EA AUG 2021
  • 出版年:   2021

▎ 摘  要

Graphite crystals used to prepare graphene-based heterostructures are generally assumed to be defect free. We report here scanning tunneling microscopy results that show graphite commonly used to prepare graphene devices can contain a significant amount of native defects. Extensive scanning of the surface allows us to determine the concentration of native defects to be 6.6 x 10(8) cm(-2). We further study the effects of these native defects on the electronic properties of Bernal-stacked bilayer graphene. We observe gate-dependent intravalley scattering and successfully compare our experimental results to T-matrix-based calculations, revealing a clear carrier density dependence in the distribution of the scattering vectors. We also present a technique for evaluating the spatial distribution of short-scale scattering. Finally, we present a theoretical analysis based on the Boltzmann transport equation that predicts that the dilute native defects identified in our study are an important extrinsic source of scattering, ultimately setting the charge carrier mobility at low temperatures.