• 文献标题:   Electron-phonon coupling and electron self-energy in electron-doped graphene: Calculation of angular-resolved photoemission spectra
  • 文献类型:   Article
  • 作  者:   CALANDRA M, MAURI F
  • 作者关键词:  
  • 出版物名称:   PHYSICAL REVIEW B
  • ISSN:   1098-0121
  • 通讯作者地址:   CNRS
  • 被引频次:   111
  • DOI:   10.1103/PhysRevB.76.205411
  • 出版年:   2007

▎ 摘  要

We obtain analytical expressions for the electron self-energy and the electron-phonon coupling in electron-doped graphene using electron-phonon matrix elements extracted from density functional theory simulations. From the electron self-energies we calculate angle-resolved photoemission spectra (ARPES). We demonstrate that the measured kink at approximate to-0.2 eV from the Fermi level is actually composed of two features, one at approximate to-0.195 eV due to the twofold-degenerate E-2g mode, and a second one at approximate to-0.16 eV due to the A(1)(') mode. The electron-phonon coupling extracted from the kink observed in ARPES experiments is roughly a factor of 5.5 larger than the calculated one. This disagreement can be only partially reconciled by the inclusion of resolution effects. Indeed, we show that a finite resolution increases the apparent electron-phonon coupling by underestimating the renormalization of the electron velocity at energies larger than the kink positions. The discrepancy between theory and experiments is thus reduced to a factor of approximate to 2.5. From the linewidth of the calculated ARPES we obtain the electron relaxation time. A comparison with available experimental data in graphene shows that the electron relaxation time detected in ARPES is almost two orders of magnitudes smaller than that measured by other experimental techniques.