• 文献标题:   Synthesis and characterization of nitrogen-doped TiO2 coatings on reduced graphene oxide for enhancing the visible light photocatalytic activity
  • 文献类型:   Article
  • 作  者:   ZHANG YF, YANG HM, PARK SJ
  • 作者关键词:   nitrogendoped tio2, reduced graphene oxide, sonochemical synthesi, solvothermal proces, visible light irradiation
  • 出版物名称:   CURRENT APPLIED PHYSICS
  • ISSN:   1567-1739 EI 1878-1675
  • 通讯作者地址:   Inha Univ
  • 被引频次:   5
  • DOI:   10.1016/j.cap.2017.12.001
  • 出版年:   2018

▎ 摘  要

Nitrogen-doped TiO2 coatings on reduced graphene oxide were prepared via a sonochemical synthesis and hydrothermal process. The nanocomposites showed improved photocatalytic activity due to their large specific surface areas (185-447 m(2)/g), the presence of TiO2 in the anatase phase, and a quenched photoluminescence peak. In particular, GN3-TiO2 (nitrogen-doped TiO2 coatings on rGO with 3 ml of titanium (IV) isopropoxide) exhibited the best photocatalytic efficiency and degradation rate among the materials prepared. With nitrogen-doped on the reduced graphene oxide surface, the photocatalytic activity is enhanced approximately 17.8 times compared to that of the pristine TiO2. The dramatic enhancement of activity is attributed to the nitrogen contents and rGO effectively promoting charge-separation efficiency and providing abundant catalytically active sites to enhance the reactivity. The composites also showed improved pollutant adsorption capacity, electronehole pair lifetime, light absorption capability, and absorbance of visible light. (C) 2017 Elsevier B.V. All rights reserved.