• 文献标题:   Interlayer Charge Transfer and Photodetection Efficiency of Graphene-Transition-Metal-Dichalcogenide Heterostructures
  • 文献类型:   Article
  • 作  者:   PARAPPURATH A, MITRA S, SINGH G, GILL NK, AHMED T, SAI TP, WATANABE K, TANIGUCHI T, GHOSH A
  • 作者关键词:  
  • 出版物名称:   PHYSICAL REVIEW APPLIED
  • ISSN:   2331-7019
  • 通讯作者地址:  
  • 被引频次:   5
  • DOI:   10.1103/PhysRevApplied.17.064062
  • 出版年:   2022

▎ 摘  要

Graphene and transition-metal-dichalcogenide-(TMD) based van der Waals heterostructures in field-effect-transistor (FET) architecture exhibits extremely high sensitivity to optical radiation due to transit and physical separation of the photogenerated carriers across the heterointerface. Both the sensitivity and speed of these detectors depend on the kinetics of charge transfer, but their interdependency at room temperature (T), where these detectors would be most useful, remains largely unexplored. Here we system-atically measure the T dependence of the magnitude (gain) and timescale (bandwidth) of photoresponse in graphene-TMD heterostructures well up to the room T. The gain-bandwidth product is found to be strongly dependent on the power of optical illumination and increases with decreasing power (P), becom-ing as large as 1 MHz in the low -P limit. We find that thermally activated back transfer of charge from graphene to the TMD determines the response time of the detector at higher temperatures under continu-ous illumination. Our experiment reveals the impact of charge-transfer pathways on the performance in a broad class of graphene-TMD detectors.