• 文献标题:   Highly sensitive and selective Love mode surface acoustic wave ammonia sensor based on graphene oxides operated at room temperature
  • 文献类型:   Article
  • 作  者:   TANG QB, GUO YJ, TANG YL, LONG GD, WANG JL, LI DJ, ZU XT, MA JY, WANG L, TORUN H, FU YQ
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF MATERIALS SCIENCE
  • ISSN:   0022-2461 EI 1573-4803
  • 通讯作者地址:   Univ Elect Sci Technol China
  • 被引频次:   2
  • DOI:   10.1007/s10853-019-03764-6
  • 出版年:   2019

▎ 摘  要

It is crucial to develop highly sensitive and selective sensors for ammonia, one of the most common toxic gases which have been widely used in pharmaceutical, chemical, and manufacturing industries. In this study, graphene oxide (GO) film was spin-coated onto surfaces of ST-cut quartz surface acoustic wave (SAW) devices with a resonant frequency of 200MHz for ammonia sensing. The oxygen-containing functional groups (such as hydroxyl and epoxy ones) on the surface of GO film strongly absorb ammonia molecules and thus increase the film stiffness. This is attributed to the main ammonia sensing mechanism of the Love mode SAW devices, which show not only a positive frequency shift of 620Hz for 500ppb ammonia gas, but also an excellent selectivity (as compared to other gases such as H-2, H2S, CO, and NO2) and a good reproducibility, operated at room temperature of 22 degrees C.