▎ 摘　　要

In the present study, low defect density graphene nanosheets (GNs) have been synthesized via chemical reduction of exfoliated graphite (EG) in the presence of a green reducing agent, oxalic acid. EG has been synthesized via chemical intercalation of natural flake graphite followed by exfoliation through microwave irradiation at 800 W for 50 s. 50 mg/mL concentration of oxalic acid helps to extract low defect density GNs from EG. As-synthesized GNs have been characterized by X-ray diffraction, Raman spectroscopy, Fourier transform infrared spectroscopy, UV-Visible spectroscopy, field emission scanning electron microscopy, and X-ray photon spectroscopy. Raman analysis confirms the removal of oxygen functional groups from EG and achieved an I-D/I-G ratio of similar to 0.10 with low defect density (similar to 1.12 x 10(10) cm(-2)). Elemental analysis supports the Raman signature of the removal of oxygen functionalities from EG, and a high C/O ratio of similar to 15.97 is obtained. Further, transparent conducting films (TCFs) have been fabricated by spray coating. The optical and electrical properties of fabricated TCFs have been measured after thermal graphitization. Thermal graphitization helps to improve the optical and electrical properties of TCFs by tuning the optical bandgap in a controlled way. TCF shows best performance when the film is annealed at 900 degrees C for 1 h in vacuum. It shows a sheet resistance of similar to 1.10 k Omega/square and a transmittance of similar to 71.56% at 550 nm. Published by AIP Publishing.