• 文献标题:   Optical Kerr effect in graphene: Theoretical analysis of the optical heterodyne detection technique
  • 文献类型:   Article
  • 作  者:   SAVOSTIANOVA NA, MIKHAILOV SA
  • 作者关键词:  
  • 出版物名称:   PHYSICAL REVIEW B
  • ISSN:   2469-9950 EI 2469-9969
  • 通讯作者地址:   Univ Augsburg
  • 被引频次:   7
  • DOI:   10.1103/PhysRevB.97.165424
  • 出版年:   2018

▎ 摘  要

Graphene is an atomically thin two-dimensional material demonstrating strong optical nonlinearities, including harmonics generation, four-wave mixing, Kerr, and other nonlinear effects. In this paper we theoretically analyze the optical heterodyne detection (OHD) technique of measuring the optical Kerr effect (OKE) in two-dimensional crystals and show how to relate the quantities measured in such experiments with components of the third-order conductivity tensor sigma((3))(alpha beta gamma delta)(omega(1)omega(2)omega(3)) of the two-dimensional crystal. Using results of a recently developed quantum theory of the third-order nonlinear electrodynamic response of graphene, we analyze the frequency, charge carrier density, temperature, and other dependencies of the OHD-OKE response of this material. We compare our results with a recent OHD-OKE experiment in graphene and find good agreement between the theory and experiment.