• 文献标题:   Fundamental limits to graphene plasmonics
  • 文献类型:   Article
  • 作  者:   NI GX, MCLEOD AS, SUN Z, WANG L, XIONG L, POST KW, SUNKU SS, JIANG BY, HONE J, DEAN CR, FOGLER MM, BASOV DN
  • 作者关键词:  
  • 出版物名称:   NATURE
  • ISSN:   0028-0836 EI 1476-4687
  • 通讯作者地址:   Columbia Univ
  • 被引频次:   98
  • DOI:   10.1038/s41586-018-0136-9
  • 出版年:   2018

▎ 摘  要

Plasmon polaritons are hybrid excitations of light and mobile electrons that can confine the energy of long-wavelength radiation at the nanoscale. Plasmon polaritons may enable many enigmatic quantum effects, including lasing(1), topological protection(2,3) and dipole-forbidden absorption(4). A necessary condition for realizing such phenomena is a long plasmonic lifetime, which is notoriously difficult to achieve for highly confined modes(5). Plasmon polaritons in graphene-hybrids of Dirac quasiparticles and infrared photons-provide a platform for exploring light-matter interaction at the nanoscale(6,7). However, plasmonic dissipation in graphene is substantial(8) and its fundamental limits remain undetermined. Here we use nanometre-scale infrared imaging to investigate propagating plasmon polaritons in high-mobility encapsulated graphene at cryogenic temperatures. In this regime, the propagation of plasmon polaritons is primarily restricted by the dielectric losses of the encapsulated layers, with a minor contribution from electron-phonon interactions. At liquid-nitrogen temperatures, the intrinsic plasmonic propagation length can exceed 10 micrometres, or 50 plasmonic wavelengths, thus setting a record for highly confined and tunable polariton modes. Our nanoscale imaging results reveal the physics of plasmonic dissipation and will be instrumental in mitigating such losses in heterostructure engineering applications.