• 文献标题:   Dye-Sensitization-Induced Visible-Light Reduction of Graphene Oxide for the Enhanced TiO2 Photocatalytic Performance
  • 文献类型:   Article
  • 作  者:   WANG P, WANG J, MING TS, WANG XF, YU HG, YU JG, WANG YG, LEI M
  • 作者关键词:   graphene, tio2rgo, photocatalysi, dyesensitizationinduced, interface
  • 出版物名称:   ACS APPLIED MATERIALS INTERFACES
  • ISSN:   1944-8244 EI 1944-8252
  • 通讯作者地址:   Wuhan Univ Technol
  • 被引频次:   108
  • DOI:   10.1021/am4008566
  • 出版年:   2013

▎ 摘  要

The reduction of graphene oxide (GO) with a large-scale production has been demonstrated to be one of the key steps for the preparation of graphene-based composite materials with various potential applications. Therefore, it is highly required to develop a facile, green, and environmentally friendly route for the effective reduction of GO. In this study, a new and effective reduced method of GO nanosheets, based on the dye-sensitization-induced visible-light reduction mechanism, was developed to prepare reduced GO (rGO) and graphene-based TiO2 composite in the absence of any additional reducing agents. It was found that the dye-sensitization-induced reduction process of GO was accompanied with the formation of TiO2-rGO composite nanostructure. The photocatalytic experimental results indicated that the resultant TiO2-rGO nanocomposites exhibited significantly higher photocatalytic performance than pure TiO2 because of a rapid separation of photogenerated electrons and holes by the rGO cocatalyst.