• 文献标题:   Plasmonically Enhanced Colloidal Quantum Dot/Graphene Doped Polymer Random Lasers
  • 文献类型:   Article
  • 作  者:   CAO MX, WANG M, WANG ZW, ZANG LH, LIU H, XIAO SP, YUEN MMF, WANG Y, ZHANG YT, YAO JQ
  • 作者关键词:   colloidal quantum dot, random laser, graphene, surface plasmon resonance
  • 出版物名称:   MATERIALS
  • ISSN:  
  • 通讯作者地址:  
  • 被引频次:   0
  • DOI:   10.3390/ma15062213
  • 出版年:   2022

▎ 摘  要

An improvement in random lasers based on a colloidal quantum dot (QD)/graphene-doped polymer was observed and attributed to multiple light-scattering and graphene surface plasmon resonance. The emission characteristics of quantum dots doped with graphene oxide and reduced graphene oxide were compared. The QD/reduced graphene oxide hybrid exhibited a lower laser emission threshold (similar to 460 mu J/cm(2)). The emission modes and thresholds were strongly dependent on both the graphene doping concentration and the external temperature. Decreased plasmon coupling was the primary reason for lower QD/graphene laser emission with increasing temperature. The optimum reduced graphene oxide concentration was 0.2 wt.%. This work provides a practical approach to optimizing the threshold and stability of random laser devices, with potential applications in displays, sensors, and anti-counterfeiting labels.