• 文献标题:   Ultrahigh solar steam generation rate of a vertically aligned reduced graphene oxide foam realized by dynamic compression
  • 文献类型:   Article
  • 作  者:   LI W, TIAN XH, LI XF, HAN S, LI CJ, ZHAI XZ, KANG Y, YU ZZ
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF MATERIALS CHEMISTRY A
  • ISSN:   2050-7488 EI 2050-7496
  • 通讯作者地址:  
  • 被引频次:   52
  • DOI:   10.1039/d1ta03014k EA JUN 2021
  • 出版年:   2021

▎ 摘  要

Although solar steam generation is a promising water purification approach for alleviating the global shortage of clean water, the water evaporation rate of non-organic systems is still far from perfection. Herein, a vertically aligned reduced graphene oxide (V-RGO) foam with numerous vertical channels is fabricated as a solar-thermal energy converter for efficient solar steam generation. For the first time, dynamic compression is proven to be an efficient strategy to adjust the energy state of water in the pore channels of V-RGO foams. With an optimal compression, the vaporization enthalpy of water significantly decreases because of the increased proportion of intermediate water, resulting in a much faster water evaporation rate under solar-light irradiation. The average water evaporation rate under 1-sun irradiation reaches 3.39 kg m(-2) h(-1), representing the highest value among those for inorganic materials reported previously. This dynamic compression provides a novel strategy for purification of wastewater and desalination of seawater.