• 文献标题:   Magnetoresistance and Magnetic Ordering Fingerprints in Hydrogenated Graphene
  • 文献类型:   Article
  • 作  者:   SORIANO D, LECONTE N, ORDEJON P, CHARLIER JC, PALACIOS JJ, ROCHE S
  • 作者关键词:  
  • 出版物名称:   PHYSICAL REVIEW LETTERS
  • ISSN:   0031-9007
  • 通讯作者地址:   Univ Alicante
  • 被引频次:   86
  • DOI:   10.1103/PhysRevLett.107.016602
  • 出版年:   2011

▎ 摘  要

Spin-dependent features in the conductivity of graphene, chemically modified by a random distribution of hydrogen adatoms, are explored theoretically. The spin effects are taken into account using a mean-field self-consistent Hubbard model derived from first-principles calculations. A Kubo transport methodology is used to compute the spin-dependent transport fingerprints of weakly hydrogenated graphene-based systems with realistic sizes. Conductivity responses are obtained for paramagnetic, antiferromagnetic, or ferromagnetic macroscopic states, constructed from the mean-field solutions obtained for small graphene supercells. Magnetoresistance signals up to similar to 7% are calculated for hydrogen densities around 0.25%. These theoretical results could serve as guidance for experimental observation of induced magnetism in graphene.