• 文献标题:   Universal Distance-Scaling of Nonradiative Energy Transfer to Graphene
  • 文献类型:   Article
  • 作  者:   GAUDREAU L, TIELROOIJ KJ, PRAWIROATMODJO GEDK, OSMOND J, DE ABAJO FJG, KOPPENS FHL
  • 作者关键词:   graphene, strong lightmatter interaction, nanooptic, energy transfer, molecule
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984 EI 1530-6992
  • 通讯作者地址:   Inst Photon Sci
  • 被引频次:   116
  • DOI:   10.1021/nl400176b
  • 出版年:   2013

▎ 摘  要

The near-field interaction between fluorescent emitters and graphene exhibits rich physics associated with local dipole-induced electromagnetic fields that are strongly enhanced due to the unique properties of graphene. Here, we measure emitter lifetimes as a function of emitter-graphene distance d, and find agreement with a universal scaling law, governed by the fine-structure constant. The observed energy transfer rate is in agreement with a 1/d(4) dependence that is characteristic of two-dimensional lossy media. The emitter decay rate is enhanced 90 times (energy transfer efficiency of similar to 99%) with respect to the decay in vacuum at distances d approximate to 15 nm. This high energy transfer rate is mainly due to the two-dimensionality and gapless character of the monatomic carbon layer. Graphene is thus shown to be an extraordinary energy sink, holding great potential for photodetection, energy harvesting, and nanophotonics.