• 文献标题:   Enhanced Fouling Resistance and Antibacterial Properties of Novel Graphene Oxide-Arabic Gum Polyethersulfone Membranes
  • 文献类型:   Article
  • 作  者:   NAJJAR A, SABRI S, ALGAASHANI R, KOCHKODAN V, ATIEH MA
  • 作者关键词:   graphene oxide, arabic gum, polyether sulfone, membrane, ultrafiltration, fouling, biofouling, hydrophilicity
  • 出版物名称:   APPLIED SCIENCESBASEL
  • ISSN:   2076-3417
  • 通讯作者地址:   HBKU
  • 被引频次:   6
  • DOI:   10.3390/app9030513
  • 出版年:   2019

▎ 摘  要

Membrane biofouling has proved to be a major obstacle when it comes to membrane efficiency in membrane-based water treatment. Solutions to this problem remain elusive. This study presents novel polyethersulfone (PES) membranes that are fabricated using the phase inversion method at different loadings of graphene oxide (GO) and 1 wt.% arabic gum (AG) as nanofiller and pore forming agents. Synthesized GO was examined using scanning electron microscopy (SEM) and transmission electron microscopy (TEM) for morphological studies and energy-dispersive X-ray spectroscopy (EDX) for elemental analysis. The prepared GO flakes showed a high content of oxygen-containing groups (similar to 31%). The fabricated membranes were extensively characterized, including water contact angle analysis for hydrophilicity, zeta potential measurements for surface charge, SEM, total porosity and pore size measurements. The prepared membranes underwent fouling tests using bovine serum albumin (BSA) solutions and biofouling tests using model Gram-positive (Bacillus subtilis) and Gram-negative (Escherichia coli) bacterial suspensions as well as real treated sewage effluent (TSE). The results showed that the novel PES/GO membranes possessed strong hydrophilicity and negative surface charge with an increase in porosity, pore size and water flux. The PES/GO membranes exhibited superior antibacterial action against both Gram-positive and Gram-negative bacterial species, implicating PES membranes which incorporate GO and AG as novel membranes that are capable of high antibiofouling properties with high flux.