• 文献标题:   Hybrid Graphene Quantum Dots@Graphene Foam Nanosheets for Dye-Sensitized Solar Cell Electrodes
  • 文献类型:   Article
  • 作  者:   CHANG QH, MA ZJ, WANG JZ, LI PP, YAN Y, SHI WZ, CHEN Q, HUANG YW, HUANG L
  • 作者关键词:   dyesensitized solar cell, electrocatalysi, graphene, nanomaterial, quantum dot
  • 出版物名称:   ENERGY TECHNOLOGY
  • ISSN:   2194-4288 EI 2194-4296
  • 通讯作者地址:   Harbin Inst Technol
  • 被引频次:   6
  • DOI:   10.1002/ente.201500194
  • 出版年:   2016

▎ 摘  要

A high-efficiency counter electrode (CE) consisting of zero-dimensional graphene quantum dots (GQDs)@graphene foam nanosheets (GFs) is proposed for dye-sensitized solar cells (DSSCs). In the hybrid CE, the nanometer-sized GQDs with more defect sites at the edges, provide outstanding electrocatalytic activity for the reduction of I-3(-). The high-quality GFs with high electronic conductivity act as fast electron transportation channels for facilitating the charge injection between the GQDs and the fluorinated tin oxide (FTO) substrate. The DSSC with the optimized hybrid CE exhibits an energy conversion efficiency (eta) of 9.59% with an open-circuit voltage (V-oc), short-circuit photocurrent density (J(sc)), and fill factor (FF) of 0.75V, 19.23mAcm(-2), and 66.5%, respectively.