• 文献标题:   Multiphoton excitation and high harmonic generation in rectangular graphene quantum dot
  • 文献类型:   Article
  • 作  者:   GHAZARYAN AG, SEDRAKIAN KV, MUSAYELYAN GA, MARKOSYAN TM
  • 作者关键词:   nanostructure, laser field, nonlinear dynamic, microscopic quantum theory, manybody coulomb interaction, multiphoton highharmonic, quantum dot
  • 出版物名称:   PHYSICA SCRIPTA
  • ISSN:   0031-8949 EI 1402-4896
  • 通讯作者地址:  
  • 被引频次:   0
  • DOI:   10.1088/1402-4896/acc9ed
  • 出版年:   2023

▎ 摘  要

The multiphoton excitation and high harmonic generation (HHG) processes are considered using the microscopic quantum theory of nonlinear interaction of strong coherent electromagnetic (EM) radiation with rectangular graphene quantum dot (RGQD). The dynamic Hartree-Fock approximation is developed for the consideration of the quantum dot-laser field nonlinear interaction at the nonadiabatic multiphoton excitation regime. The many-body Coulomb interaction is described in the extended Hubbard approximation. By numerical results, we show the significance of the RGQD lateral size, shape, and EM wavefield orientation in RGQD of the zigzag edge compear to the armchair edge in the HHG process allowing for increasing the cutoff photon energy and the quantum yield of higher harmonics. The differences via edge on the elongated side of the RGQD have been explained by the investigation of the dipole momentum in both cases. Numerical results have shown that the HHG spectra have a strong anisotropy depending on the orientation of the laser wave, and the cutoff photon energy shifts toward blue with an increase in the transverse size of the RGQD.