▎ 摘　　要

The electromechanical actuation of a highly ordered compound of graphene oxide (GO) is shown via ab initio simulations to produce high-performance quantum-mechanical responses, which mimic the behaviour of mammalian skeletal muscle. In addition to large expansive strains (similar to 10%), this GO compound (asymmetrically unzipped C4O) exhibits large contractive strains of -4.8% upon -0.15 e/C-atom electron injection. Furthermore, as these contractive strains are coupled with equally high stresses (similar to 100 GPa) and short response times (similar to 1 ns), we show that this GO material meets all of the functional requirements of an artificial muscle building block. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4775597]