▎ 摘　　要

A facile and cost-effective preparation of moisture-responsive graphene bilayer paper by focused sunlight irradiation is reported. The smart graphene paper shows moisture-responsive properties due to selective adsorption of water molecules, leading to controllable actuation under humid conditions. In this way, graphene-based moisture-responsive actuators including a smart claw, an orientable transporter, and a crawler paper robot are successfully developed.