• 文献标题:   Controlled doping of graphene by impurity charge compensation via a polarized ferroelectric polymer
  • 文献类型:   Article
  • 作  者:   FIGUEROA KS, PINTO NJ, MANDYAM SV, ZHAO MQ, WEN CY, DAS PM, GAO ZL, DRNDIC M, JOHNSON ATC
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF APPLIED PHYSICS
  • ISSN:   0021-8979 EI 1089-7550
  • 通讯作者地址:   Univ Puerto Rico
  • 被引频次:   1
  • DOI:   10.1063/5.0003099
  • 出版年:   2020

▎ 摘  要

A simple technique of doping graphene by manipulating adsorbed impurity charges is presented. Using a field effect transistor configuration, controlled polarization of a ferroelectric polymer gate is used to compensate and neutralize charges of one type. The uncompensated charges of the opposite type then dope graphene. Both n- and p-type doping are possible by this method, which is non-destructive and reversible. We observe a change in n-type dopant concentration of 8x10(12)cm(-2) and a change in electron mobility of 650%. The electron and hole mobilities are inversely proportional to the impurity concentration, as predicted by theory. Selective doping of graphene can be achieved using this method by patterning gate electrodes at strategic locations and programming them independently. Such charge control without introducing hard junctions, therefore, permits seamless integration of multiple devices on a continuous graphene film.