• 文献标题:   Seeing Many-Body Effects in Single- and Few-Layer Graphene: Observation of Two-Dimensional Saddle-Point Excitons
  • 文献类型:   Article
  • 作  者:   MAK KF, SHAN J, HEINZ TF
  • 作者关键词:  
  • 出版物名称:   PHYSICAL REVIEW LETTERS
  • ISSN:   0031-9007 EI 1079-7114
  • 通讯作者地址:   Columbia Univ
  • 被引频次:   261
  • DOI:   10.1103/PhysRevLett.106.046401
  • 出版年:   2011

▎ 摘  要

Significant excitonic effects were observed in graphene by measuring its optical conductivity in a broad spectral range including the two-dimensional pi-band saddle-point singularities in the electronic structure. The strong electron-hole interactions manifest themselves in an asymmetric resonance peaked at 4.62 eV, which is redshifted by nearly 600 meV from the value predicted by ab initio GW calculations for the band-to-band transitions. The observed excitonic resonance is explained within a phenomenological model as a Fano interference of a strongly coupled excitonic state and a band continuum. Our experiment also showed a weak dependence of the excitonic resonance in few-layer graphene on layer thickness. This result reflects the effective cancellation of the increasingly screened repulsive electron-electron (e-e) and attractive electron-hole (e-h) interactions.