• 文献标题:   Time-resolved energy transfer from single chloride-terminated nanocrystals to graphene
  • 文献类型:   Article
  • 作  者:   AJAYI OA, ANDERSON NC, COTLET M, PETRONE N, GU T, WOLCOTT A, GESUELE F, HONE J, OWEN JS, WONG CW
  • 作者关键词:  
  • 出版物名称:   APPLIED PHYSICS LETTERS
  • ISSN:   0003-6951 EI 1077-3118
  • 通讯作者地址:   Columbia Univ
  • 被引频次:   18
  • DOI:   10.1063/1.4874298
  • 出版年:   2014

▎ 摘  要

We examine the time-resolved resonance energy transfer of excitons from single n-butyl amine-bound, chloride-terminated nanocrystals to two-dimensional graphene through time-correlated single photon counting. The radiative biexponential lifetime kinetics and blinking statistics of the individual surface-modified nanocrystal elucidate the non-radiative decay channels. Blinking modification as well as a 4 x reduction in spontaneous emission were observed with the short chloride and n-butylamine ligands, probing the energy transfer pathways for the development of graphene-nanocrystal nanophotonic devices. (C) 2014 AIP Publishing LLC.