• 文献标题:   A universal growth strategy for DNA-programmed quantum dots on graphene oxide surfaces
  • 文献类型:   Article
  • 作  者:   WANG JD, GAO ZH, HE SQ, JIN PH, MA DQ, GAO YB, WANG LB, HAN SM
  • 作者关键词:   quantum dot, graphene oxide, dna, graphene based nanomaterial, twodimensional material
  • 出版物名称:   NANOTECHNOLOGY
  • ISSN:   0957-4484 EI 1361-6528
  • 通讯作者地址:   Yanshan Univ
  • 被引频次:   1
  • DOI:   10.1088/1361-6528/ab7c42
  • 出版年:   2020

▎ 摘  要

The emerging materials of semiconductor quantum dots/graphene oxide (QDs/GO) hybrid composites have recently attracted intensive attention in materials science and technology due to their potential applications in electronic and photonic devices. Here, a simple and universal strategy to produce DNA-programmed semiconductor quantum dots/graphene oxide (QDs/GO) hybrid composites with controllable sizes, shapes, compositions, and surface properties is reported. This proof-of-concept work successfully demonstrates the use of sulfhydryl modified single-stranded DNA (S-ssDNA) as a 'universal glue' which can adsorb onto GO easily and provide the growth sites to synthesize CdS QDs, CdSe QDs, CdTe QDs and CdTeSe QDs with distinctive sizes, shapes and properties. Also, adapting this method, other graphene oxide-based hybrid materials which are easily synthesized in aqueous solution, including oxides, core-shell structure QDs and metal nanocrystals, would be possible. This method provided a universal strategy for the synthesis and functional realization of graphene -based nanomaterials.