• 文献标题:   Gram-Scale Synthesis of Porous Graphene via Printing Paper Pyrolysis as Supercapacitor Electrodes
  • 文献类型:   Article
  • 作  者:   WANG M, LIU CY, ALBOLKANY MK, ZHAO MM, ZHU CF, LIU B
  • 作者关键词:   graphene, high power density, largescale synthesi, printing paper, supercapacitor
  • 出版物名称:   ENERGY TECHNOLOGY
  • ISSN:   2194-4288 EI 2194-4296
  • 通讯作者地址:  
  • 被引频次:   3
  • DOI:   10.1002/ente.202001025 EA APR 2021
  • 出版年:   2021

▎ 摘  要

Graphene has great potential in the application as supercapacitor electrode materials owing to its unique properties. However, it is challenging to find a facile and cost-efficient method using cheap raw materials for large-scale synthesis. Herein, a simple method is demonstrated for converting printing paper to graphene via one-step pyrolysis followed by washing. Various characterizations are used to analyze the obtained samples, revealing the typical graphene feature of the products. The sample obtained at 900 degrees C (denoted as G-900) shows a specific surface area of 514 m(2) g(-1) with a 50% mesopore volume. The symmetric supercapacitor using G-900 as an active electrode material gives rise to an ultrahigh power density of 49 kW kg(-1) at a high current density of 10 A g(-1), along with a great specific capacitance of 164.4 F g(-1). The capacitance retention ratio is as high as 93% after cycling for 4000 cycles at a current density of 1 A g(-1). As hundreds of million tons of paper are used annually, converting the waste paper to graphene is a scalable way for practical applications, associated with the facile conversion procedures.