• 文献标题:   Reduced Graphene Oxide Thin Film with Strong Optical Nonlinearity
  • 文献类型:   Article, Early Access
  • 作  者:   HEIDARI B, GHAMSARI MS, SALMANI S, AHMADI M, MAJLESARA MH
  • 作者关键词:   reduced graphene oxide, saturable absorber, strong optical nonlinearity, thin film, z #8208, scan
  • 出版物名称:   PHYSICA STATUS SOLIDI BBASIC SOLID STATE PHYSICS
  • ISSN:   0370-1972 EI 1521-3951
  • 通讯作者地址:   Kharazmi Univ
  • 被引频次:   0
  • DOI:   10.1002/pssb.202000397 EA DEC 2020
  • 出版年:  

▎ 摘  要

Herein, a simple, low-cost, and scalable process is developed to prepare the reduced graphene oxide (rGO) thin films (TFs) with strong optical nonlinearity. To do so, a chemical reduction method (using inorganic agent hydroiodic acid) and drop-casting technique are used. Optical nonlinearity of the prepared thin rGO film is measured by the Z-scan technique at low light intensity (continuous-wave wavelength of 632 nm). The result of optical nonlinearity responses is illustrated by a remarkable nonlinear refraction index (n(2) approximate to 10(-4) cm(2) W-1) as well as a considerable nonlinear absorption coefficient (beta = 1.43 x 10(-8) cm(2) W-1) compared with similar reported results. Moreover, experimental results show that the prepared film enjoys a positive nonlinear refractive index with strong optical nonlinearity. Results also confirm that the changes made in optical absorption of rGO TFs are due to state filling effects and the optical nonlinearity proportional to the carriers' density is in fact due to thermal effects of SiO2 substrate.