• 文献标题:   Heterostructured graphene quantum dot/WSe2/Si photodetector with suppressed dark current and improved detectivity
  • 文献类型:   Article
  • 作  者:   SUN MX, FANG QY, XIE D, SUN YL, QIAN L, XU JL, XIAO P, TENG CJ, LI WW, REN TL, ZHANG YF
  • 作者关键词:   heterojunction, photodetector, si, wse2, graphene quantum dot
  • 出版物名称:   NANO RESEARCH
  • ISSN:   1998-0124 EI 1998-0000
  • 通讯作者地址:   Tsinghua Univ
  • 被引频次:   6
  • DOI:   10.1007/s12274-017-1855-1
  • 出版年:   2018

▎ 摘  要

A high-performance heterojunction photodetector is formed by combining an n-type Si substrate with p-type monolayer WSe2 obtained using physical vapor deposition. The high quality of the WSe2/Si heterojunction is demonstrated by the suppressed dark current of 1 nA and the extremely high rectification ratio of 10(7). Under illumination, the heterojunction exhibits a wide photoresponse range from ultraviolet to near-infrared radiation. The introduction of graphene quantum dots (GQDs) greatly elevates the photodetective capabilities of the heterojunction with strong light absorption and long carrier lifetimes. The GQDs/WSe2/Si heterojunction exhibits a high responsivity of 707 mA center dot W-1, short response time of 0.2 ms, and good specific detectivity of 4.51 x 10(9) Jones. These properties suggest that the GQDs/WSe2/Si heterojunction holds great potential for application in future high-performance photodetectors.