• 文献标题:   All-two-dimensional semitransparent and flexible photodetectors employing graphene/MoS2/graphene vertical heterostructures
  • 文献类型:   Article
  • 作  者:   KO JS, SHIN DH, LEE WJ, JANG CW, KIM S, CHOI SH
  • 作者关键词:   twodimensional, graphene, doping, mos2, photodetector, semitransparent, flexible, vertical, heterostructure
  • 出版物名称:   JOURNAL OF ALLOYS COMPOUNDS
  • ISSN:   0925-8388 EI 1873-4669
  • 通讯作者地址:  
  • 被引频次:   17
  • DOI:   10.1016/j.jallcom.2020.158118 EA MAR 2021
  • 出版年:   2021

▎ 摘  要

As human society develops, electronic/optoelectronic devices are further required to be foldable, wearable, and even visually comfortable, but simultaneous achievement of both performance and comfort is a tough task. Here, we first report all-two-dimensional (2D) bis (trifluoromethanesulfonyl)-amide (TFSA)-doped graphene (GR) (TFSA-GR)/MoS2/ triethylene tetramine (TETA)-doped GR (TETA-GR) vertical-heterostructure semitransparent photodetectors (PDs) on rigid flexible substrates. The PD exhibits 0.128 A/W responsivity (R) and 1.69 x 10(9) cm Hz(1/)(2)/W detectivity at 532 nm wavelength with average visible transmittance being 58%. By adding an Al reflective mirror to the semitransparent PD, the R is improved to 0.137 A/W. The unencapsulated PD maintains similar to 75% of its initial R under 25 degrees C/30% relative humidity for 1000 h. The flexible PD shows excellent bending stability by maintaining 32% of its initial R even after 2000 bending cycles at a radius of curvature of 2 mm. These results suggest that the all-2D TFSA-GR/MoS2/TETA-GR vertical heterostructures are very promising for their applications in flexible, foldable, and/or semitransparent electronic/optoelectronic appliances. (C) 2020 Elsevier B.V. All rights reserved.