• 文献标题:   Exchange interactions and frustrated magnetism in single-side hydrogenated and fluorinated graphene
  • 文献类型:   Article
  • 作  者:   RUDENKO AN, KEIL FJ, KATSNELSON MI, LICHTENSTEIN AI
  • 作者关键词:  
  • 出版物名称:   PHYSICAL REVIEW B
  • ISSN:   1098-0121
  • 通讯作者地址:   Hamburg Univ Technol
  • 被引频次:   31
  • DOI:   10.1103/PhysRevB.88.081405
  • 出版年:   2013

▎ 摘  要

Magnetism in single-side hydrogenated (C2H) and fluorinated (C2F) graphene is analyzed in terms of the Heisenberg model with parameters determined from first principles. We predict a frustrated ground state for both systems, which means the instability of collinear spin structures and sheds light on the absence of a conventional magnetic ordering in defective graphene demonstrated in recent experiments. Moreover, our findings suggest a highly correlated magnetic behavior at low temperatures offering the possibility of a spin-liquid state.