▎ 摘　　要

Pt catalysts with nitrogen-doped graphene oxide (GO) as support and CeO2 as promoter were prepared by impregnation method, and their catalytic oxidation of formaldehyde (HCHO) at room temperature was tested. The Pt-CeO2/N-rGO (reduced GO) with a mass fraction of 0.7% Pt and 0.8% CeO2 exhibited an excellent catalytic performance with the 100% conversion of HCHO at room temperature. Physicochemical characterization demonstrated that nitrogen doping greatly increased the defect degree and the specific surface area of GO, enhanced the dispersion of Pt and promoted more zero-valent Pt. The synergistic effect between CeO2 and Pt was also beneficial to the dispersion of Pt. Nitrogen-doping promoted the production of more Ce3+ ions, generating more oxygen vacancies, which was conducive to O-2 adsorption. As a result, the catalyst exhibited enhanced redox properties, leading to the best catalytic activity. Finally, an attempt to propose the reaction mechanism of HCHO oxidation has been made. (c) 2022 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.