• 文献标题:   Ultrathin sub-3 nm nitrogen-doped graphene quantum dot layers coated TiO2 nanocomposites as high-performance photocatalysts
  • 文献类型:   Article
  • 作  者:   KIM S, CHANG H, CHOI JY, SONG Y, HELLER MJ
  • 作者关键词:  
  • 出版物名称:   CHEMICAL PHYSICS LETTERS
  • ISSN:   0009-2614 EI 1873-4448
  • 通讯作者地址:   Univ Calif San Diego
  • 被引频次:   6
  • DOI:   10.1016/j.cplett.2018.10.058
  • 出版年:   2019

▎ 摘  要

We introduce a facile fabrication process for ultrathin nitrogen-doped graphene quantum dot (NGQD) layers on TiO2 nanoparticles in order to develop high-performance photocatalysts. NGQDs are grown either by graphitization of precursors or direct deposition of premade NGQDs. Photocatalytic performance is shown to be dependent on the thickness of NGQD layers and doping levels of C and N atoms on TiO2 surfaces. The nanocomposites shown to absorb a broad range of visible light and narrow the bandgap by 0.38 eV, resulting in the increased density of photoinduced eletron-hole pairs and efficient charge separation at the interface between the NGQDs and TiO2.