• 文献标题:   Perovskite/Poly(3-hexylthiophene)/Graphene Multiheterojunction Phototransistors with Ultrahigh Gain in Broadband Wavelength Region
  • 文献类型:   Article
  • 作  者:   XIE C, YAN F
  • 作者关键词:   phototransistor, perovskite, graphene, responsivity, hole transport layer
  • 出版物名称:   ACS APPLIED MATERIALS INTERFACES
  • ISSN:   1944-8244 EI 1944-8252
  • 通讯作者地址:   Hong Kong Polytech Univ
  • 被引频次:   46
  • DOI:   10.1021/acsami.6b11631
  • 出版年:   2017

▎ 摘  要

Organometal halide perovskite materials have attracted much attention recently for then. excellent optoelectronic properties. Here, we report an ultrasensitive photo transistor based on the multiheterojunction of CH3NH3PbI3-xClx perovskite/poly(3-hexylthiophene)/graphene for the first time. Since the photoexcited electrons and: holes are effectively separated by the poly(3-hexylthiophene)layer, high-density electrons are trapped in the perovskite layer, leading to a strong photogating effect on the underlying graphene channel. The phototransistor demonstrates an unprecedented ultrahigh responsivity of similar to 4.3 X 10(9) A/W and a gain approaching 10(10) electrons per photon, respectively. More importantly, the device is sensitive in a broadband wavelength region from ultraviolet to near-infrared, which has not yet been achieved with other perovskite photodetectors. It is expected that the novel: perovskite phototransistor will find promising applications as photodetection and imaging devices in the future.