• 文献标题:   Adsorption and removal of rhodamine B from aqueous solution by tannic acid functionalized graphene
  • 文献类型:   Article
  • 作  者:   LIU KP, LI HM, WANG YM, GOU XJ, DUAN YX
  • 作者关键词:   graphene, tannic acid, rhodamine b, adsorption kinetic
  • 出版物名称:   COLLOIDS SURFACES APHYSICOCHEMICAL ENGINEERING ASPECTS
  • ISSN:   0927-7757 EI 1873-4359
  • 通讯作者地址:   Sichuan Univ
  • 被引频次:   64
  • DOI:   10.1016/j.colsurfa.2015.03.048
  • 出版年:   2015

▎ 摘  要

A facile and green method was employed to synthesize the tannic acid functionalized graphene nanocomposite (TA-G) using tannic acid as reducing as well as capping reagent which could alter graphene surface physicochemical properties to improve the adsorption efficiency. Then the as-prepared TA-G was used as adsorbent to investigate the adsorption behavior for rhodamine B (RB). Due to the intensive pi-pi stacking interaction and electrostatic attraction, TA-G exhibited fine adsorption performance for RB. The adsorption isotherm fitted Langmuir model well and the theoretical maximum of adsorption capacity calculated by Langmuir model was 201 mg g(-1) which was approximately in a close agreement with the experimental measured data. The kinetics of adsorption was consistent with the pseudo-second-order model perfectly and chemisorption was the speed limit step. Therefore, the as-prepared TA-G nanocomposite would be an ideal adsorbent for the removal of RB in aqueous solution and opened a new door to broaden the potential applications of graphene in environmental research. (C) 2015 Elsevier B.V. All rights reserved.