• 文献标题:   Sulfur-doped graphitic carbon nitride decorated with graphene quantum dots for an efficient metal-free electrocatalyst
  • 文献类型:   Article
  • 作  者:   XU CY, HAN Q, ZHAO Y, WANG LX, LI Y, QU LT
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF MATERIALS CHEMISTRY A
  • ISSN:   2050-7488 EI 2050-7496
  • 通讯作者地址:   Beijing Inst Technol
  • 被引频次:   112
  • DOI:   10.1039/c4ta06149g
  • 出版年:   2015

▎ 摘  要

A rationally designed strategy has been developed for spontaneous reduction and assembly of graphene quantum dots rich in carbonyl and carboxylic groups (ox-GQDs) onto sulfur doped graphitic carbon nitride (s-g-C3N4) nanosheets to form unique s-g-C3N4@GQD nanohybrids by a one-step hydrothermal treatment. The fabricated architectures exhibit remarkably enhanced catalytic activity in the oxygen reduction reaction far better than the original s-g-C3N4 and GQDs, which is even comparable to those of well-developed graphene and GQD-based catalysts, demonstrating the potential towards energy conversion applications.