• 文献标题:   Role of Remote Interfacial Phonon (RIP) Scattering in Heat Transport Across Graphene/SiO2 Interfaces
  • 文献类型:   Article
  • 作  者:   KOH YK, LYONS AS, BAE MH, HUANG B, DORGAN VE, CAHILL DG, POP E
  • 作者关键词:   remote interfacial phonon rip seattering, graphene interface, interfaces of 2d material, interfacial thermal conductance, electrostatic pressure, electrostatic control of heat conduction
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984 EI 1530-6992
  • 通讯作者地址:   Natl Univ Singapore
  • 被引频次:   14
  • DOI:   10.1021/acs.nanolett.6b01709
  • 出版年:   2016

▎ 摘  要

heat transfer across interfaces of graphene and polar dielectrics (e.g.; SiO2) could be Mediated by direct: phonon coupling, as well as electronic coupling with remote interfacial phonons (RIPs). To understand-the relative contribution of each component, we develop a new pump probe technique called voltage-modulated thermorefleetance (VMTR) to accurately measure the change-of interfacial: thermal conductance under an electrostatic field. We employed VMTR on top gates of graphene field-,effect-transistors. and find that the thermal conductance of SiO2/graphene/SiO2 interfaces increases by up to Delta G approximate to 0.8 MW M-2 K-1 under electrostatic fields of <0.2 V nm(-1). We propose two possible explanations for-the small observed Delta G. First, because the applied electrostatic field induces charge carriers in graphene, out VMTR measurements could originate from heat transfer-between the charge carriers in graphene and RIPs in SiO2. Second, the increase in heat conduction could be caused by better conformity of graphene interfaces under electrostatic pressure exerted by the induced charge carriers. Regardless of the origins of the observed Delta G, our VMTR measurements eStablish, an upper limit for heat transfer from unbiased graphene to SiO2 substrates via RIP scattering; for example, only <2% of the interfacial heat transport is facilitated' y RIP scattering even at a carrier concentration of similar to 4 X 10(12) cm(-2).