• 文献标题:   Z-Scheme MoS2/TiO2/graphene nanohybrid photocatalysts for visible light-induced degradation for highly efficient water disinfection and antibacterial activity
  • 文献类型:   Article
  • 作  者:   CHEN L, HUANG CP, CHUANG Y, NGUYEN TB, CHEN CW, DONG CD
  • 作者关键词:  
  • 出版物名称:   NEW JOURNAL OF CHEMISTRY
  • ISSN:   1144-0546 EI 1369-9261
  • 通讯作者地址:  
  • 被引频次:   3
  • DOI:   10.1039/d2nj01824a EA JUL 2022
  • 出版年:   2022

▎ 摘  要

We fabricated MoS2/TiO2/graphene (MTG) nanohybrids using a hydrothermal process in the preparation of heterostructure photocatalysts. The MTG nanohybrids exhibited high stability, large specific surface area, and visible light response. The heterostructure nanohybrids were effective in the visible-light photodegradation of tetracycline (TC), rhodamine B (RhB), and congo red (CR), as well as Pb(ii) reduction. The nanohybrids exhibited a photocatalytic TC removal capability of 94.5% with 60 min of visible light irradiation. Suppressing the recombination of photoexcited electron-hole pairs enhanced the removal of environmental pollutants. The MTG nanohybrids also displayed photocatalytic reduction of Pb(ii), approximately 10-15 times that of bare MoS2 and TiO2 samples. The nanohybrids also showed efficient photocatalytic antibacterial performance, killing 99.9% of E. coli in 10 min, thus demonstrating environmental friendliness in water disinfection. The results clearly demonstrated promising nanohybrids for the photocatalytic removal of a wide variety of contaminants, such as hazardous organic chemicals, heavy metals, and pathogenic microbes, under visible light irradiation.