• 文献标题:   N, S-doped Graphene Quantum Dots Grafted Graphitic Carbon Nitride to Boost its Photocatalytic Hydrogen Evolution and Antibacterial Activity
  • 文献类型:   Article
  • 作  者:   LI JL, LIU HL, BAI X, RAO X, ZHANG YP
  • 作者关键词:   graphitic carbon nitride, n sdoped graphene quantum dots n sgqds, photocatalysi, antibacterial activity
  • 出版物名称:   NANO
  • ISSN:   1793-2920 EI 1793-7094
  • 通讯作者地址:  
  • 被引频次:   0
  • DOI:   10.1142/S1793292022500667 EA SEP 2022
  • 出版年:   2022

▎ 摘  要

Constructing heterojunction is one promising strategy to improve the transfer and separation of photoinduced charge carriers of graphitic carbon nitride (CN). Herein, nonmetal N, S-doped graphene quantum dots (N, S-GQDs)/g-C3N4 nanocomposite photocatalysts were successfully synthesized by calcining N, S-GQDs (NSGs) and melamine at elevated temperature. The optimal 06NSG-CN composite effectively reduced the concentration of Escherichia coli flora under visible light irradiation by superoxide and super hydroxyl radicals. Meanwhile, the optimum photocatalytic hydrogen evolution reaches 50.9 mu mol/h, about 16.9 times that of pure phase CN under visible light. Graphitic carbon nitride (g-C3N4) grafted with N, S-doped GQDs could increase the specific surface area, promote the absorption and utilization of visible light, and inhibited the recombination of photoinduced electron-hole pairs, resulting in excellent photocatalytic antibacterial activity.