• 文献标题:   Highly stable electrocatalysts supported on nitrogen-self-doped three-dimensional graphene-like networks with hierarchical porous structures
  • 文献类型:   Article
  • 作  者:   CHENG JH, LI YY, HUANG XD, WANG QQ, MEI A, SHEN PK
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF MATERIALS CHEMISTRY A
  • ISSN:   2050-7488 EI 2050-7496
  • 通讯作者地址:   Sun Yat Sen Univ
  • 被引频次:   19
  • DOI:   10.1039/c4ta05552g
  • 出版年:   2015

▎ 摘  要

The nitrogen-self-doped three-dimensional graphene-like networks (N-3D GNs) with suitable surface areas and hierarchical porous structures have been synthesized by an improved ion-exchange/activation method. The Pt nanoparticles supported on N-3D GNs give more than double mass activity and almost no degradation in surface area after 5000 cycles compared with a commercial Pt/C catalyst. The results demonstrate that the improvement in the support can reach 2.6 times the catalytic activity. This strategy is a direct way to reduce the catalyst cost and make the practical application of the catalyst a reality.