• 文献标题:   Excitonic Fano Resonance in Free-Standing Graphene
  • 文献类型:   Article
  • 作  者:   CHAE DH, UTIKAL T, WEISENBURGER S, GIESSEN H, VON KLITZING K, LIPPITZ M, SMET J
  • 作者关键词:   suspended graphene, exciton, spectroscopy, fano resonance
  • 出版物名称:   NANO LETTERS
  • ISSN:   1530-6984
  • 通讯作者地址:   Max Planck Inst Solid State Res
  • 被引频次:   88
  • DOI:   10.1021/nl200040q
  • 出版年:   2011

▎ 摘  要

We investigate the role of electron-hole correlations in the absorption of free-standing monolayer and bilayer graphene using optical transmission spectroscopy from 1.5 to 5.5 eV. Line shape analysis demonstrates that the ultraviolet region is dominated by an asymmetric Fano resonance. We attribute this to an excitonic resonance that forms near the van Hove singularity at the saddle point of the band structure and couples to the Dirac continuum. The Fano model quantitatively describes the experimental data all the way down to the infrared. In contrast, the common noninteracting particle picture cannot describe our data. These results suggest a profound connection between the absorption properties and the topology of the graphene band structure.