• 文献标题:   Graphene Decorated with Silver Nanoparticles as a Low Temperature Methane Gas Sensor
  • 文献类型:   Article
  • 作  者:   GHANBARI R, SAFAIEE R, SHEIKHI MH, GOLSHAN MM, HORASTANI ZK
  • 作者关键词:   decorated graphene, silver nanoparticle, methane sensor, low temperature, humidity
  • 出版物名称:   ACS APPLIED MATERIALS INTERFACES
  • ISSN:   1944-8244 EI 1944-8252
  • 通讯作者地址:   Shiraz Univ
  • 被引频次:   10
  • DOI:   10.1021/acsami.9b00625
  • 出版年:   2019

▎ 摘  要

This paper is devoted to an investigation on the methane sensing properties of graphene (G), decorated with silver nanoparticles (AgNPs), under ambient conditions. To do so, we first present an effective modification in the standard manner of decorating graphene by AgNPs. From structural analysis of the product (AgNPs/G), it is concluded that graphene is indeed decorated by AgNPs of a mean size 29.3 nm, free of aggregation, with a uniform distribution. The so produced material is then used, as a resistivity-based sensor, to examine its response to the presence of methane gas. Our measurements are performed at relatively low temperatures, for various silver-to-graphene mass ratios (SGMRs) and methane concentrations. To account for the effects of humidity, we have made the measurements, at room temperature, for different levels of humidity. Our results demonstrate that an increase in the SGMR enhances the response of AgNPs/G to methane with an optimum value of SGMR congruent to 12% It is also illustrated that for methahe concentrations less than 2000 ppm, the maximal response increases linearly and rapidly, even at room temperature. Moreover, we demonstrate that AgNPs/G is of low limit of detection, highly stable, selective, reversible, repeatable, and sensor-to-sensor reproducible, for methane sensing. The results thus promise a low-cost and simple-to-fabricate methane device.