• 文献标题:   Removal of bisphenol A over a separation free 3D Ag3PO4-graphene hydrogel via an adsorption-photocatalysis synergy
  • 文献类型:   Article
  • 作  者:   MU CF, ZHANG Y, CUI WQ, LIANG YH, ZHU YF
  • 作者关键词:   ag3po4/rgh hydrogel, 3d structure, adsorptionphotocatalysi, bpa removal
  • 出版物名称:   APPLIED CATALYSIS BENVIRONMENTAL
  • ISSN:   0926-3373 EI 1873-3883
  • 通讯作者地址:   North China Univ Sci Technol
  • 被引频次:   82
  • DOI:   10.1016/j.apcatb.2017.04.018
  • 出版年:   2017

▎ 摘  要

Here we reported a silver phosphate/graphene hydrogel (Ag3PO4/rGH) with efficient degradation of bisphenol A (BPA) with the synergy of adsorption and photocatalysis. The Ag3PO4/rGH 3D structure exhibits enriched adsorption-photocatalytic degradation ability for the removal of BPA under visible light irradiation, and its three-dimensional structure facilitates the rapid recycle and reuse ability of the photocatalyst. The maximum adsorption capacity was 15 mg/g which is 2.1 times and 2.4 times than that of Ag3PO4/AC, Ag3PO4/Al2O3. The BPA could be even 100% removed in 12 min by the synergy of adsorption and photocatalysis under visible light irradiation. The removal ability was more than 90% after recycling 5 time indicating superiority of separation freely without complicated filter system for 3D structured hydrogel. The Ag3PO4/rGH 3D structure also showed high removal activity and stability in the continuous flow reaction system, and the 100% removal of BPA have been maintained more than 60 h. In all, Ag3PO4/rGH 3D structure possesses superiority of separation freely without complicated filter system. (C) 2017 Elsevier B.V. All rights reserved.