• 文献标题:   Graphene-Based Materials for Hydrogen Generation from Light-Driven Water Splitting
  • 文献类型:   Review
  • 作  者:   XIE GC, ZHANG K, GUO BD, LIU Q, FANG L, GONG JR
  • 作者关键词:   graphene, hydrogen generation, water splitting, photocatalysi, photoelectrochemistry
  • 出版物名称:   ADVANCED MATERIALS
  • ISSN:   0935-9648 EI 1521-4095
  • 通讯作者地址:   Natl Ctr Nanosci Technol
  • 被引频次:   415
  • DOI:   10.1002/adma.201301207
  • 出版年:   2013

▎ 摘  要

Hydrogen production from solar water splitting has been considered as an ultimate solution to the energy and environmental issues. Over the past few years, graphene has made great contribution to improving the light-driven hydrogen generation performance. This article provides a comprehensive overview of the recent research progress on graphene-based materials for hydrogen evolution from light-driven water splitting. It begins with a brief introduction of the current status and basic principles of hydrogen generation from solar water splitting, and tailoring properties of graphene for application in this area. Then, the roles of graphene in hydrogen generation reaction, including an electron acceptor and transporter, a cocatalyst, a photocatalyst, and a photosensitizer, are elaborated respectively. After that, the comparison between graphene and other carbon materials in solar water splitting is made. Last, this review is concluded with remarks on some challenges and perspectives in this emerging field.