• 文献标题:   Ultrafast spectroscopic imaging of exfoliated graphene
  • 文献类型:   Article
  • 作  者:   GRANCINI G, MARTINO N, BIANCHI M, RIZZI LG, RUSSO V, LI BASSI A, CASARI CS, PETROZZA A, SORDAN R, LANZANI G
  • 作者关键词:   carriers cooling, graphene, transient absorption imaging, ultrafast dynamic
  • 出版物名称:   PHYSICA STATUS SOLIDI BBASIC SOLID STATE PHYSICS
  • ISSN:   0370-1972
  • 通讯作者地址:   Ist Italiano Tecnol
  • 被引频次:   4
  • DOI:   10.1002/pssb.201200108
  • 出版年:   2012

▎ 摘  要

In this paper we investigate the carrier cooling dynamics in graphene flakes exploiting ultrafast transient absorption imaging technique. This tool enables us to combine nanoscale spatial resolution and sub-picosecond (ps) time resolution. It provides many advantages over the standard transient absorption techniques because it directly investigates the excited state dynamics at a local scale that would be usually averaged out. The local dynamics show a photobleaching recovery in the first ps, assigned to cooling by electronphonon scattering. We found that the photoexcited carrier dynamics is spatially uniform over the micrometer-sized exfoliated graphene layer. Ultrafast pumpprobe technique is combined with an optical microscope to investigate the local excited state dynamics in graphene flakes.