• 文献标题:   Improved trade-off between thermoelectric performance and mechanical reliability of Mg2Si by hybridization of few-layered reduced graphene oxides
  • 文献类型:   Article
  • 作  者:   KIM G, KIM SW, RIM HJ, LEE H, KIM J, ROH JW, KIM BW, LEE KH, LEE W
  • 作者关键词:   nanocomposite, thermoelectric, mg2si, reduced graphene oxide, fracture toughnes
  • 出版物名称:   SCRIPTA MATERIALIA
  • ISSN:   1359-6462
  • 通讯作者地址:   Yonsei Univ
  • 被引频次:   7
  • DOI:   10.1016/j.scriptamat.2018.11.052
  • 出版年:   2019

▎ 摘  要

Nanocomposites can simultaneously enhance the thermoelectric and mechanical properties of thermoelectric materials. Here, we fabricated bulks of Mg1.96Al0.04Si0.97Bi0.03 with monodispersed few-layered reduced graphene oxides utilizing ultrasonic-based wet chemical pulverizing-mixing and spark plasma sintering to improve unfavorable trade-off between thermoelectric performance and mechanical reliability, which is important for commercialization. An unexpected high fracture toughness of similar to 1.88 MPa m(1/2) was observed due to the synergetic effect of the deflection of crack propagation, bridging, and sheet pull-out mechanisms, and a high thermoelectric figure of merit similar to 0.6 was obtained even for a high content (3 vol.%) of reduced graphene oxides. (C) 2018 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.