• 文献标题:   High performance CsPbBr3 perovskite nanocrystal vertical phototransistor with graphene electrode
  • 文献类型:   Article
  • 作  者:   CHE YL, CAO XL, ZHANG YT, YAO JQ
  • 作者关键词:   vertical phototransistor, perovskite nanocrystal, graphene electrode
  • 出版物名称:   OPTICAL MATERIALS
  • ISSN:   0925-3467 EI 1873-1252
  • 通讯作者地址:   Shandong Univ Sci Technol
  • 被引频次:   1
  • DOI:   10.1016/j.optmat.2020.109664
  • 出版年:   2020

▎ 摘  要

All-inorganic cesium lead halide perovskites (CsPbX3, X = Cl, Br, and I) nanocrystals (NCs) have been extensively studied as optically active materials in photodetectors, light-emitting diodes, solar cells and lasers, in view of their combination of the outstanding characteristics of perovskites and NCs such as low cost, solution processability, bandgap tunability, and large absorption coefficient. Here we report the fabrication of graphene electrode based CsPbBr3 NCs vertical field-effect phototransistor (VFEPT), exhibiting high photoelectrical performances benifiting from the ultrashort channel, the high ultraviolet visible absorption of CsPbBr3 NCs, and the adjustable Fermi level of graphene. The VFEPT exhibited high drain current density of 0.25 A/cm(2) for p-type and 0.2 A/cm(2) for n-type transports in dark condition. The responsivity, effective quantum efficiency and detectivity reached as high as 2.2 x 10(3) A/W, 6.7 x 10(5)%, 1.1 x 10(9) Jones at an irradiance power of 342 mW/cm(2) under 405 nm illumination. Additionally, the device showed excellent stable and reproducible dynamic response to cyclical optical signal, with the rise and decay time as fast as 20 ms/36 ms. The device described here has great potential applications in high-sensitivity, high-speed, and low-power nanometer-scale photodetectors.