• 文献标题:   Enhanced photocatalytic activity of multifunctional graphene quantum dots decorated TiO2 film for dye-sensitized solar cells
  • 文献类型:   Article
  • 作  者:   FAN TJ, JIAN LF, HUANG XW, ZHANG SY, MURTAZA I, ABID R, LIU YD, MIN YG
  • 作者关键词:  
  • 出版物名称:   JOURNAL OF MATERIALS SCIENCEMATERIALS IN ELECTRONICS
  • ISSN:   0957-4522 EI 1573-482X
  • 通讯作者地址:  
  • 被引频次:   2
  • DOI:   10.1007/s10854-022-09023-w EA SEP 2022
  • 出版年:   2022

▎ 摘  要

Graphene quantum dots, as one of the pioneering materials applied in energy storage devices, possess outstanding electrical, optical, thermal, and mechanical properties. Concerning the commercial application of dye-sensitized solar cells, it is imperative to seek materials with highly effective photocatalytic activity. Herein, a novel carbon-based material based on graphene quantum dot nanorods has been prepared via hydrothermal treatment in addition to the syntheses of graphene quantum dots (GQDs) with sizes of approximately 5 and 20 nm. Efficient photoelectrodes are fabricated based on graphene quantum dot nanorods (GQDs-NRs) decorated TiO2 and their use in dye-sensitized solar cells (DSSCs) is successfully demonstrated with the maximum short circuit current density of 18.20 +/- 0.02 mA cm(-2) and an efficiency of 8.06 +/- 0.01%, which are remarkably greater than even traditional DSSCs (without GQDs). Hence, incorporating GQDs-NRs and GQDs with controllable size not only enhances dye-sensitized solar cell properties but also decreases the amount of dye or colorant required, which is significant for cost reduction and environmental protection. Thus, the present work provides a practical approach for configuring the size of GQDs-NRs and original GQDs for their onward utilization in TiO2-coated electrodes. The synthesized material shows high photocatalytic activity, making it suitable for efficient and cost-effective energy transformation devices.