• 文献标题:   Regulation and enhancement of the nonlinear optical properties of reduced graphene oxide through Au nanospheres and Au@CdS core-shells
  • 文献类型:   Article
  • 作  者:   HAO Y, WANG LW, ZHU BH, ZHANG YM, GU YZ
  • 作者关键词:  
  • 出版物名称:   OPTICS EXPRESS
  • ISSN:   1094-4087
  • 通讯作者地址:  
  • 被引频次:   11
  • DOI:   10.1364/OE.422584
  • 出版年:   2021

▎ 摘  要

Regulating nonlinear optical (NLO) absorption and refraction properties of graphene is significant in nonlinear photonics. In this work, the functionalizing strategy of quantum dots (QDs) was used for the regulation of the NLO properties of reduced graphene oxide (rGO) with Au nanospheres and Au@CdS core-shells. The third-order NLO properties of rGO-Au and rGO-Au@CdS nanocomposites were investigated by Z-scan technique with 38 ps laser pulses at 532 nm wavelength. The saturation absorption (SA) of rGO was weakened when it was combined with Au nanospheres and switched to reverse saturation absorption (RSA) when combined with Au@CdS core-shells as irradiance intensity increased. The strength of RSA was tunable with the size of Au@CdS core-shells. Meanwhile, the nonlinear susceptibility of rGO was weakened with the complex Au but was tunable with the complex Au@CdS and realized two times enhancement. The effect of charge transfer mechanism was proposed to explain the regulated effect. (C) 2021 Optical Society of America under the terms of the OSA Open Access Publishing Agreement