• 文献标题:   Forest-like Laser-Induced Graphene Film with Ultrahigh Solar Energy Utilization Efficiency
  • 文献类型:   Article
  • 作  者:   PENG YY, ZHAO WW, NI F, YU WJ, LIU XQ
  • 作者关键词:   forestlike laserinduced graphene, broadband light absorbance, photothermal material, photothermal actuator, saltrejecting desalination
  • 出版物名称:   ACS NANO
  • ISSN:   1936-0851 EI 1936-086X
  • 通讯作者地址:  
  • 被引频次:   44
  • DOI:   10.1021/acsnano.1c06277
  • 出版年:   2021

▎ 摘  要

To achieve high solar energy utilization efficiency, photothermal materials with broadband absorption of sunlight and high conversion efficiency are becoming a fast-growing research focus. Inspired by the forest structure with efficient sunlight utilization, we designed and fabricated a graphene film consisting of densely arranged porous graphene though laser scribing on polybenzoxazine resin (poly(Ph-ddm)). This hierarchical structure significantly reduced the light reflection of graphene as a 2D material. With a combination of advanced photothermal conversion properties of graphene, the 3D structured graphene film, named forest-like laser-induced graphene (forest-like LIG), was endowed with a very high light absorption of 99.0% over the whole wavelength range of sunlight as well as advanced light-to-heat conversion performance (reaching up to 87.7 degrees C within 30 s under the illumination of simulated sunlight and showing an equilibrium temperature of 90.7 +/- 0.4 degrees C). As a further benefit of its superhydrophobicity, a photothermal actuator with quick actuated response and high motion velocity, as well as a solar-driven interfacial desalination membrane with durable salt-rejecting properties and high solar evaporation efficiencies, was demonstrated.