• 文献标题:   Effect of reduction time on third order optical nonlinearity of reduced graphene oxide
  • 文献类型:   Article
  • 作  者:   SREEJA VG, VINITHA G, RESHMI R, ANILA EI, JAYARAJ MK
  • 作者关键词:   reduced graphene oxide, z scan technique, nonlinear absorption coefficient, saturable absorption, saturation intensity, nonlinear refractive index
  • 出版物名称:   OPTICAL MATERIALS
  • ISSN:   0925-3467 EI 1873-1252
  • 通讯作者地址:   Union Christian Coll
  • 被引频次:   13
  • DOI:   10.1016/j.optmat.2017.01.042
  • 出版年:   2017

▎ 摘  要

We report the influence of reduction time on structural, linear and nonlinear optical properties of reduced graphene oxide (rGO) thin films synthesized by spin coating method. We observed that the structural, linear and nonlinear optical properties can be tuned with reduction time in GO is due to the increased structural ordering because of the restoration of sp2 carbon atoms with the time of reduction. The nonlinear absorption studies by open aperture Z-scan technique exhibited a saturable absorption. The nonlinear refraction studies showed the self de focusing nature of rGO by closed aperture Z scan technique. The nonlinear absorption coefficient and saturation intensity varies with the time for reduction of GO which is attributed to the depletion of valence band and the conduction band filling effect. Our results emphasize duration for reduction of GO dependent optical nonlinearity of rGO thin films to a great extent and explore its applications Q switched mode locking laser systems for generating ultra short laser pulses and in optical sensors. The rGO coated films were characterized by X-Ray diffraction method (XRD), Fourier transform infrared spectroscopy (FTIR), Raman spectroscopy, UV Vis absorption spectroscopy (UV Vis), Photoluminescence (PL) and Scanning electron microscope (SEM) measurements. (C) 2017 Elsevier B.V. All rights reserved.