• 文献标题:   Large Scale Graphene/Hexagonal Boron Nitride Heterostructure for Tunable Plasmonics
  • 文献类型:   Article
  • 作  者:   ZHANG K, YAP FL, LI K, NG CT, LI LJ, LOH KP
  • 作者关键词:   hexagonal boron nitride, graphene, plasma chemical vapor deposition, heterostructure, plasmon
  • 出版物名称:   ADVANCED FUNCTIONAL MATERIALS
  • ISSN:   1616-301X EI 1616-3028
  • 通讯作者地址:   Natl Univ Singapore
  • 被引频次:   42
  • DOI:   10.1002/adfm.201302009
  • 出版年:   2014

▎ 摘  要

Vertical integration of hexagonal boron nitride (h-BN) and graphene for the fabrication of vertical field-effect transistors or tunneling diodes has stimulated intense interest recently due to the enhanced performance offered by combining an ultrathin dielectric with a semi-metallic system. Wafer scale fabrication and processing of these heterostructures is needed to make large scale integrated circuitry. In this work, by using remote discharged, radio-frequency plasma chemical vapor deposition, wafer scale, high quality few layer h-BN films are successfully grown. By using few layer h-BN films as top gate dielectric material, the plasmon energy of graphene can be tuned by electrostatic doping. An array of graphene/h-BN vertically stacked micrometer-sized disks is fabricated by lithography and transfer techniques, and infrared spectroscopy is used to observe the modes of tunable graphene plasmonic absorption as a function of the repeating (G/h-BN)(n) units in the vertical stack. Interestingly, the plasmonic resonances can be tuned to higher frequencies with increasing layer thickness of the disks, showing that such vertical stacking provides a viable strategy to provide wide window tuning of the plasmons beyond the limitation of the monolayer.