• 文献标题:   Simultaneous Photoreduction and Nitrogen Doping of Graphene Oxide for Supercapacitors by Direct Laser Writing
  • 文献类型:   Article
  • 作  者:   FU XY, XU S, LUO Y, LI AW, YANG H
  • 作者关键词:   simultaneous photoreduction nitrogendoping, graphene based supercapacitor, direct laser writing
  • 出版物名称:   CHEMICAL RESEARCH IN CHINESE UNIVERSITIES
  • ISSN:   1005-9040 EI 2210-3171
  • 通讯作者地址:   Jilin Univ
  • 被引频次:   2
  • DOI:   10.1007/s40242-019-9060-2
  • 出版年:   2019

▎ 摘  要

Graphene-based supercapacitors have attracted tremendous attention owing to their outstanding electro-chemical performance. In terms of material, nitrogen(N)-doped graphene(NDG) displays enhanced specific capaci- tance and rate performance compared with bare graphene used as a supercapacitor electrode. However, it still remains a challenge to develop a facile and simple method of NDG in cost-effective manner. Here, we used a simple direct laser writing technique to accomplish the simultaneous photoreduction and N-doping of graphene oxide(GO) using urea as a N source. The N content of the resultant reduced N-doped graphene oxide(NGO) reached a maximum value of 6.37%. All reduced NGO(NRGO)-based supercapacitors exhibited a higher specific capacitance than those based on pure reduced GO(RGO). Interestingly, the electrochemical performance of NRGO-based supercapacitors varied with different contents of N species. Therefore, we can control the properties of the obtained NRGOs by adjusting the doping ratios, an important step in developing effective graphene-based energy storage devices.